A method includes the following steps. An original carbon nanotube film is provided. The original carbon nanotube film includes a plurality of carbon nanotubes substantially oriented along a first direction. The original carbon nanotube film is suspended. The suspended original carbon nanotube film is soaked with an atomized organic solvent to shrink into a carbon nanotube film. Wherein the atomized organic solvent comprises a plurality of dispersed organic droplets with diameters of larger than or equal to 10 micrometers, and less than or equal to 100 micrometers.