A method for producing a crystallographically oriented ceramic including a preparation step of preparing a template layer having uniform crystal orientation in a predetermined direction, a formation step of forming a shaped body including a matrix layer arranged on the template layer, the matrix layer being composed of a mixed material that contains a lead-containing material and an additional material containing lithium and boron, and a firing step of firing the shaped body formed in the formation step at a predetermined firing temperature. Furthermore, after the firing step, a post-annealing step of heating the shaped body to remove lithium and boron may be included.