A process method for bond-packaging an LED using a thermoplastic resin photoconverter by rolling includes at least the following continuous process flow: preparation of a photoconversion sheet, shaping and cutting of a photoconversion sheet array, forming of LED package elements by roll-bonding, and curing of the LED package elements. The present invention has a significant advantage of bond-packaging the LED by continuous rolling, can meet a condition requirement of bond-packaging the LED using the thermoplastic resin photoconverter, and can enhance the production efficiency and yield of LED packages in industrialized batch production.