Embodiments of the present disclosure provide a method and a device for controlling an electronic device, and a computer-readable storage medium. The method includes: receiving a preset instruction; activating a second camera when controlling a first camera to capture a first image of a first field of view; controlling the second camera to capture a second image of a second field of view, in which the second field of view is different from or not exactly the same with the first field of view; and storing the first image and the second image, and establishing a correspondence between the first image and the second image.