Simplified methods for preparing a catalyst coated membrane (CCM) for solid polymer electrolyte fuel cells. The CCM has two reinforcing, expanded polymer sheets and the methods involve forming the electrolyte membrane from ionomer solution during assembly of the CCM. Thus, the conventional requirement to obtain, handle, and decal transfer solid polymer sheets in CCM preparation can be omitted. Further, CCM structures with improved mechanical strength can be prepared by orienting the expanded polymer sheets such that the stronger tensile strength direction of one is orthogonal to the other. Such improved CCM structures can be fabricated using the simplified methods.